Advanced Materials in Catalysis by Frank Bolz (Auth.)

By Frank Bolz (Auth.)

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Chem. 74, 216. Holt, E. (1964). Nature 203, 857. Innes, W. B. (1954). In "Catalysis" (P. H. ). Vol. I, pp. 2 4 5 - 3 1 4 , Reinhold, New York. Kilty, P. , and Sachtler, W. M. H. (1974). Catal. —Set. Eng. 10(1), 1. Kokes, R. , and Emmett, P. H. (1959). J. Am. Chem. Soc. 8 1 , 5032. Kulifay, S. M, (1962). J. Am. Chem. Soc. 83, 4916. Lytic, F. W. (1965a). In "Physics of Non-Crystalline Solids" (J. A. ), p. 12. , Amsterdam. Lytic, F. W. (1965b). In "Advances in X-ray Analysis," (G. R. Mallett, M. Fay, and W.

J. Catal. 16, 220. Cant, N . , and Hall, W. K. (1972). J. Catal. 27, 70. Carter, J. , Cusumano, J. , and Sinfelt, J. H. (1971). / . Catal. 20, 223. 30 J . Η. S i n f e l t a n d J . A. C u s u m a n o Ciapetta, F. , and Plank, C. J. (1954). In "Catalysis" (P. H. ), Vol. I, pp. 3 1 5 - 3 5 2 . Reinhold, New York. Cusumano, J. A. (1974). S. Pat. N o . 3,844,981. Cusumano, J. , Dembinski, G. , and Sinfelt, J. H. (1966). J. Catal. 5, 471. Dekker, A . J . (1957). "Solid State Physics," pp. 104-111. Prentice-Hall, Englewood Cliflfs, New Jersey.

Diagram looks like Fig. ) The application of this rule to real phase diagrams is straight forward. Figure 13 is a typical phase diagram—that of the silver/gold system. At the silver-rich side of the diagram, the melting curve looks like Fig. 12a, and n o segregation of Au to the surface of Ag is expected. At the gold-rich side of the diagram the melting curve looks like Fig. 12b, and segregation of Ag to the surface of Au is expected. Experimentally, Overbury and Somorjai (1976) have shown that Au does not segregate to the surface of Ag but Ag does segregate to the surface of Au (Nelson, 1976), as predicted.

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